Time-resolved pump-probe spectroscopy of intraband absorption by a semiconductor nanorod

Mikhail Yu Leonov, Ivan D. Rukhlenko, Alexander V Baranov, Anatoly V Fedorov

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Abstract

We develop a theory of time-resolved pump-probe optical spectroscopy of intraband absorption of a probe pulse inside an anisotropic semiconductor nanorod. The absorption is preceded by the absorption of the pump pulse resonant to an interband transition. It is assumed that the resonantly exited states of the nanorod are interrelated via the relaxation induced by their interaction with a bath. We reveal the conditions for which the absorption of the probe's pulse is governed by a simple formula regardless of the pulse's shape. This formula is useful for the analysis of the experimental data containing information on the relaxation parameters of the nanorod's electronic subsystem.

Original languageEnglish
Title of host publicationNanophotonic Materials X
EditorsStefano Cabrini , Gilles Lérondel, Adam M. Schwartzberg, Taleb Mokari
PublisherSPIE
Number of pages10
Volume8807
ISBN (Print)9780819496577
DOIs
Publication statusPublished - 2013
EventNanophotonic Materials X 2013 - San Diego, United States of America
Duration: 28 Aug 201329 Aug 2013
http://spie.org/Publications/Proceedings/Volume/8807?SSO=1
https://www.spiedigitallibrary.org/conference-proceedings-of-spie/8807.toc (Proceedings of SPIE)

Publication series

NameSPIE - International Society for Optical Engineering. Proceedings
PublisherS P I E - International Society for Optical Engineering
ISSN (Print)0277-786X
ISSN (Electronic)1996-756X

Conference

ConferenceNanophotonic Materials X 2013
CountryUnited States of America
CitySan Diego
Period28/08/1329/08/13
OtherProceedings Volume 8807,
Nanophotonic Materials X; 880701 (2013);
doi: 10.1117/12.2034132
Event: SPIE NanoScience + Engineering, 2013, San Diego, California, United States
Internet address

Keywords

  • Pump-probe spectroscopy
  • Relaxation parameters
  • Semiconductor nanorod
  • Transient intraband absorption

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