High-Mobility Ambipolar Organic Thin-Film Transistor Processed from a Nonchlorinated Solvent

Prashant Sonar; Jingjing Chang; Jae H. Kim; Kok Haw Ong; Eliot Gann; Sergei Manzhos; Jishan Wu; Christopher R. McNeill

doi:10.1021/acsami.6b08075

High-Mobility Ambipolar Organic Thin-Film Transistor Processed from a Nonchlorinated Solvent

Prashant Sonar
, Jingjing Chang
, Jae H. Kim
, Kok Haw Ong
, Eliot Gann
, Sergei Manzhos
, Jishan Wu
, Christopher R. McNeill

Materials Science & Engineering

Research output: Contribution to journal › Article › Research › peer-review

33 Citations (Scopus)

Abstract

Polymer semiconductor PDPPF-DFT, which combines furan-substituted diketopyrrolopyrrole (DPP) and a 3,4-difluorothiophene base, has been designed and synthesized. PDPPF-DFT polymer semiconductor thin film processed from nonchlorinated hexane is used as an active layer in thin-film transistors. As a result, balanced hole and electron mobilities of 0.26 and 0.12 cm²/(V s) are achieved for PDPPF-DFT. This is the first report of using nonchlorinated hexane solvent for fabricating high-performance ambipolar thin-film transistor devices.

Original language	English
Pages (from-to)	24325-24330
Number of pages	6
Journal	ACS Applied Materials & Interfaces
Volume	8
Issue number	37
DOIs	https://doi.org/10.1021/acsami.6b08075
Publication status	Published - 21 Sept 2016

Keywords

ambipolar transistors
balanced charge carrier mobilities
difluorothiophene
diketopyrrolopyrrole
nonchlorinated solvent
polymer semiconductors

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10.1021/acsami.6b08075

Cite this

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title = "High-Mobility Ambipolar Organic Thin-Film Transistor Processed from a Nonchlorinated Solvent",

abstract = "Polymer semiconductor PDPPF-DFT, which combines furan-substituted diketopyrrolopyrrole (DPP) and a 3,4-difluorothiophene base, has been designed and synthesized. PDPPF-DFT polymer semiconductor thin film processed from nonchlorinated hexane is used as an active layer in thin-film transistors. As a result, balanced hole and electron mobilities of 0.26 and 0.12 cm2/(V s) are achieved for PDPPF-DFT. This is the first report of using nonchlorinated hexane solvent for fabricating high-performance ambipolar thin-film transistor devices.",

keywords = "ambipolar transistors, balanced charge carrier mobilities, difluorothiophene, diketopyrrolopyrrole, nonchlorinated solvent, polymer semiconductors",

author = "Prashant Sonar and Jingjing Chang and Kim, \{Jae H.\} and Ong, \{Kok Haw\} and Eliot Gann and Sergei Manzhos and Jishan Wu and McNeill, \{Christopher R.\}",

year = "2016",

month = sep,

day = "21",

doi = "10.1021/acsami.6b08075",

language = "English",

volume = "8",

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journal = "ACS Applied Materials \& Interfaces",

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T1 - High-Mobility Ambipolar Organic Thin-Film Transistor Processed from a Nonchlorinated Solvent

AU - Sonar, Prashant

AU - Chang, Jingjing

AU - Kim, Jae H.

AU - Ong, Kok Haw

AU - Gann, Eliot

AU - Manzhos, Sergei

AU - Wu, Jishan

AU - McNeill, Christopher R.

PY - 2016/9/21

Y1 - 2016/9/21

N2 - Polymer semiconductor PDPPF-DFT, which combines furan-substituted diketopyrrolopyrrole (DPP) and a 3,4-difluorothiophene base, has been designed and synthesized. PDPPF-DFT polymer semiconductor thin film processed from nonchlorinated hexane is used as an active layer in thin-film transistors. As a result, balanced hole and electron mobilities of 0.26 and 0.12 cm2/(V s) are achieved for PDPPF-DFT. This is the first report of using nonchlorinated hexane solvent for fabricating high-performance ambipolar thin-film transistor devices.

AB - Polymer semiconductor PDPPF-DFT, which combines furan-substituted diketopyrrolopyrrole (DPP) and a 3,4-difluorothiophene base, has been designed and synthesized. PDPPF-DFT polymer semiconductor thin film processed from nonchlorinated hexane is used as an active layer in thin-film transistors. As a result, balanced hole and electron mobilities of 0.26 and 0.12 cm2/(V s) are achieved for PDPPF-DFT. This is the first report of using nonchlorinated hexane solvent for fabricating high-performance ambipolar thin-film transistor devices.

KW - ambipolar transistors

KW - balanced charge carrier mobilities

KW - difluorothiophene

KW - diketopyrrolopyrrole

KW - nonchlorinated solvent

KW - polymer semiconductors

UR - https://www.scopus.com/pages/publications/84988649045

U2 - 10.1021/acsami.6b08075

DO - 10.1021/acsami.6b08075

M3 - Article

AN - SCOPUS:84988649045

SN - 1944-8244

VL - 8

SP - 24325

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JO - ACS Applied Materials & Interfaces

JF - ACS Applied Materials & Interfaces

IS - 37

ER -

High-Mobility Ambipolar Organic Thin-Film Transistor Processed from a Nonchlorinated Solvent

Abstract

Keywords

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