TY - JOUR
T1 - Efficient conversion of methane into power via microchanneled solid oxide fuel cells
AU - Wang, Jingjing
AU - Fan, Dongjie
AU - Yu, Libo
AU - Wei, Tao
AU - Hu, Xun
AU - Ye, Zhengmao
AU - Wang, Zhi
AU - Wang, Yi
AU - Li, Cuncheng
AU - Yao, Jianfeng
AU - Dong, Dehua
N1 - Funding Information:
Prof. D. H. Dong acknowledges the startup funding provided by the University of Jinan . This work is supported by the National Natural Science Foundation of China ( 51872123 ). The study is a part of the projects of Natural Science Foundation of Shandong Province ( ZR2017MEM022 ) and Shandong Province Key Research and Development Program ( 2018GGX102037 ).
Publisher Copyright:
© 2020 Elsevier B.V.
PY - 2020/3/31
Y1 - 2020/3/31
N2 - Methane-fueled solid oxide fuel cells (SOFCs) are promising to achieve high energy conversion efficiency while no study focuses on the conversion efficiency of methane into power, which is greatly restrained by gas diffusion within anode supports. This study employs microchanneled anode supports to provide fast gas diffusion pathway. To confirm the advantage, the anodes with half-channels and without channels are also used for comparison. The microchannel structure increases the maximum power density up to 2.5 times because of diminishing or eliminating concentration polarization within anode supports and improving catalyst coating over anode internal surface. As a compromise of fuel utilization and power output, methane conversion efficiency is defined as power output per mol methane input in feeding gas to compare with the reported results, and the microchanneled SOFCs achieve the record high methane conversion efficiency.
AB - Methane-fueled solid oxide fuel cells (SOFCs) are promising to achieve high energy conversion efficiency while no study focuses on the conversion efficiency of methane into power, which is greatly restrained by gas diffusion within anode supports. This study employs microchanneled anode supports to provide fast gas diffusion pathway. To confirm the advantage, the anodes with half-channels and without channels are also used for comparison. The microchannel structure increases the maximum power density up to 2.5 times because of diminishing or eliminating concentration polarization within anode supports and improving catalyst coating over anode internal surface. As a compromise of fuel utilization and power output, methane conversion efficiency is defined as power output per mol methane input in feeding gas to compare with the reported results, and the microchanneled SOFCs achieve the record high methane conversion efficiency.
KW - Anode supports
KW - Gas diffusion
KW - Methane conversion efficiency
KW - Methane-fueled SOFCs
KW - Microchannel structure
UR - http://www.scopus.com/inward/record.url?scp=85078960867&partnerID=8YFLogxK
U2 - 10.1016/j.jpowsour.2020.227848
DO - 10.1016/j.jpowsour.2020.227848
M3 - Article
AN - SCOPUS:85078960867
SN - 0378-7753
VL - 453
JO - Journal of Power Sources
JF - Journal of Power Sources
M1 - 227848
ER -