TY - JOUR
T1 - Cosmic spherules from Widerøefjellet, Sør Rondane Mountains (East Antarctica)
AU - Goderis, Steven
AU - Soens, Bastien
AU - Huber, Matthew S.
AU - McKibbin, Seann
AU - van Ginneken, Matthias
AU - Van Maldeghem, Flore
AU - Debaille, Vinciane
AU - Greenwood, Richard C.
AU - Franchi, Ian A.
AU - Cnudde, Veerle
AU - Van Malderen, Stijn
AU - Vanhaecke, Frank
AU - Koeberl, Christian
AU - Topa, Dan
AU - Claeys, Philippe
N1 - Funding Information:
This work was made possible by the 2009 Baillet Latour Antarctica Fellowship to SG. Additional support was provided by the Interuniversity Attraction Poles Program (IUAP) Planet Topers and BRAIN-be BAMM! projects initiated by the Belgian Science Policy Office and the FWO/FNRS Excellence of Science project ET-HoME (ID 30442502). SG and PhC also acknowledge continuous funding by the VUB Strategic Research Council . VD thanks the FRS-FNRS and ERC StG “ ISoSyC ” for support. FV thanks Ghent University Special Research Fun (BOF-UGent) for financial support under the form of a GOA project. SVM is a postdoctoral fellow of the FWO and acknowledges the financial and logistic support from the Research Foundation - Flanders (FWO, research project 12S5718N). All authors would like to acknowledge the Centre for X-ray Tomography at Ghent University, Belgium , for the performed experiments. VC acknowledges the Ghent University Special Research Fund (BOF-UGent) for financial support to BOF.EXP.2017.0007. Oxygen isotope studies at the Open University are funded by a consolidated grant from the Science and Technology Facilities Council, UK (STFC grant ST/P000657/1 ). The reported oxygen isotope data in this work was measured in the framework of Europlanet 2020 Research Infrastructure Transnational Access project 15-EPN-033. Europlanet 2020 RI has received funding from the European Union's Horizon 2020 research and innovation program under grant agreement No 654208. This work benefited significantly from support in the field by Alain Hubert and the International Polar Foundation. We extend our gratitude to O. Steenhaut, L. Pittarello, C. Ventura-Bordenca, T. De Kock, C. Suavet, P. Rochette, and L. Folco for their help and advice during various phases of this work. We thank Martin Suttle and 2 anonymous reviewers as well as associate editor Rhian Jones for their detailed comments and suggestions that helped to improve this manuscript significantly. Appendix A
Funding Information:
This work was made possible by the 2009 Baillet Latour Antarctica Fellowship to SG. Additional support was provided by the Interuniversity Attraction Poles Program (IUAP) Planet Topers and BRAIN-be BAMM! projects initiated by the Belgian Science Policy Office and the FWO/FNRS Excellence of Science project ET-HoME (ID 30442502). SG and PhC also acknowledge continuous funding by the VUB Strategic Research Council. VD thanks the FRS-FNRS and ERC StG ?ISoSyC? for support. FV thanks Ghent University Special Research Fun (BOF-UGent) for financial support under the form of a GOA project. SVM is a postdoctoral fellow of the FWO and acknowledges the financial and logistic support from the Research Foundation - Flanders (FWO, research project 12S5718N). All authors would like to acknowledge the Centre for X-ray Tomography at Ghent University, Belgium, for the performed experiments. VC acknowledges the Ghent University Special Research Fund (BOF-UGent) for financial support to BOF.EXP.2017.0007. Oxygen isotope studies at the Open University are funded by a consolidated grant from the Science and Technology Facilities Council, UK (STFC grant ST/P000657/1). The reported oxygen isotope data in this work was measured in the framework of Europlanet 2020 Research Infrastructure Transnational Access project 15-EPN-033. Europlanet 2020 RI has received funding from the European Union's Horizon 2020 research and innovation program under grant agreement No 654208. This work benefited significantly from support in the field by Alain Hubert and the International Polar Foundation. We extend our gratitude to O. Steenhaut, L. Pittarello, C. Ventura-Bordenca, T. De Kock, C. Suavet, P. Rochette, and L. Folco for their help and advice during various phases of this work. We thank Martin Suttle and 2 anonymous reviewers as well as associate editor Rhian Jones for their detailed comments and suggestions that helped to improve this manuscript significantly.
Publisher Copyright:
© 2019 Elsevier Ltd
PY - 2020/2/1
Y1 - 2020/2/1
N2 - A newly discovered sedimentary accumulation of micrometeorites in the Sør Rondane Mountains of East Antarctica, close to the Widerøefjellet summit at ∼2750 m above sea level, is characterized in this work. The focus here lies on 2099 melted cosmic spherules larger than 200 μm, extracted from 3.2 kg of sampled sediment. Although the Widerøefjellet deposit shares similarities to the micrometeorite traps encountered in the Transantarctic Mountains, both subtle and more distinct differences in the physicochemical properties of the retrieved extraterrestrial particles and sedimentary host deposits are discernable (e.g., types of bedrock, degree of wind exposure, abundance of metal-rich particles). Unlike the Frontier Mountain and Miller Butte sedimentary traps, the size fraction below 240 μm indicates some degree of sorting at Widerøefjellet, potentially through the redistribution by wind, preferential alteration of smaller particles, or processing biases. However, the cosmic spherules larger than 300 μm appear largely unbiased following their size distribution, frequency by textural type, and bulk chemical compositions. Based on the available bedrock exposure ages for the Sør Rondane Mountains, extraterrestrial dust is estimated to have accumulated over a time span of ∼1–3 Ma at Widerøefjellet. Consequently, the Widerøefjellet collection reflects a substantial reservoir to sample the micrometeorite influx over this time interval. Petrographic observations and 3D microscopic CT imaging are combined with chemical and triple-oxygen isotopic analyses of silicate-rich cosmic spherules larger than 325 μm. The major element composition of 49 cosmic spherules confirms their principally chondritic parentage. For 18 glassy, 15 barred olivine, and 11 cryptocrystalline cosmic spherules, trace element concentrations are also reported on. Based on comparison with evaporation experiments reported in literature and accounting for siderophile and chalcophile element losses during high-density phase segregation and ejection, the observed compositional sequence largely reflects progressive heating and evaporation during atmospheric passage accompanied by significant redox shifts, although the influence of (refractory) chondrite mineral constituents and terrestrial alteration cannot be excluded in all cases. Twenty-eight cosmic spherules larger than 325 μm analyzed for triple-oxygen isotope ratios confirm inheritance from mostly carbonaceous chondritic precursor materials (∼55% of the particles). Yet, ∼30% of the measured cosmic spherules and ∼50% of all glassy cosmic spherules are characterized by oxygen isotope ratios above the terrestrial fractionation line, implying genetic links to ordinary chondrites and parent bodies currently unsampled by meteorites. The structural, textural, chemical, and isotopic characteristics of the cosmic spherules from the Sør Rondane Mountains, and particularly the high proportion of Mg-rich glass particles contained therein, imply a well-preserved and representative new sedimentary micrometeorite collection from a previously unstudied region in East Antarctica characterized by distinct geological and exposure histories.
AB - A newly discovered sedimentary accumulation of micrometeorites in the Sør Rondane Mountains of East Antarctica, close to the Widerøefjellet summit at ∼2750 m above sea level, is characterized in this work. The focus here lies on 2099 melted cosmic spherules larger than 200 μm, extracted from 3.2 kg of sampled sediment. Although the Widerøefjellet deposit shares similarities to the micrometeorite traps encountered in the Transantarctic Mountains, both subtle and more distinct differences in the physicochemical properties of the retrieved extraterrestrial particles and sedimentary host deposits are discernable (e.g., types of bedrock, degree of wind exposure, abundance of metal-rich particles). Unlike the Frontier Mountain and Miller Butte sedimentary traps, the size fraction below 240 μm indicates some degree of sorting at Widerøefjellet, potentially through the redistribution by wind, preferential alteration of smaller particles, or processing biases. However, the cosmic spherules larger than 300 μm appear largely unbiased following their size distribution, frequency by textural type, and bulk chemical compositions. Based on the available bedrock exposure ages for the Sør Rondane Mountains, extraterrestrial dust is estimated to have accumulated over a time span of ∼1–3 Ma at Widerøefjellet. Consequently, the Widerøefjellet collection reflects a substantial reservoir to sample the micrometeorite influx over this time interval. Petrographic observations and 3D microscopic CT imaging are combined with chemical and triple-oxygen isotopic analyses of silicate-rich cosmic spherules larger than 325 μm. The major element composition of 49 cosmic spherules confirms their principally chondritic parentage. For 18 glassy, 15 barred olivine, and 11 cryptocrystalline cosmic spherules, trace element concentrations are also reported on. Based on comparison with evaporation experiments reported in literature and accounting for siderophile and chalcophile element losses during high-density phase segregation and ejection, the observed compositional sequence largely reflects progressive heating and evaporation during atmospheric passage accompanied by significant redox shifts, although the influence of (refractory) chondrite mineral constituents and terrestrial alteration cannot be excluded in all cases. Twenty-eight cosmic spherules larger than 325 μm analyzed for triple-oxygen isotope ratios confirm inheritance from mostly carbonaceous chondritic precursor materials (∼55% of the particles). Yet, ∼30% of the measured cosmic spherules and ∼50% of all glassy cosmic spherules are characterized by oxygen isotope ratios above the terrestrial fractionation line, implying genetic links to ordinary chondrites and parent bodies currently unsampled by meteorites. The structural, textural, chemical, and isotopic characteristics of the cosmic spherules from the Sør Rondane Mountains, and particularly the high proportion of Mg-rich glass particles contained therein, imply a well-preserved and representative new sedimentary micrometeorite collection from a previously unstudied region in East Antarctica characterized by distinct geological and exposure histories.
KW - Atmospheric heating
KW - Cosmic spherules
KW - Extraterrestrial dust
KW - Oxygen isotope ratios
KW - Parent bodies
UR - http://www.scopus.com/inward/record.url?scp=85076044758&partnerID=8YFLogxK
U2 - 10.1016/j.gca.2019.11.016
DO - 10.1016/j.gca.2019.11.016
M3 - Article
AN - SCOPUS:85076044758
SN - 0016-7037
VL - 270
SP - 112
EP - 143
JO - Geochimica et Cosmochimica Acta
JF - Geochimica et Cosmochimica Acta
ER -