TY - JOUR
T1 - Comparison and modeling of leachate transportation dominated by the field permeability with an anisotropic characteristic based on a large-scale field trial study
AU - Yin, Ke
AU - Chan, Wei-Ping
AU - Dou, Xiaomin
AU - Lisak, Grzegorz
AU - Wei-Chung Chang, Victor
PY - 2020/3
Y1 - 2020/3
N2 - Permeability significantly affects leachate transportation. Yet, there often exists a gap for its measurements between laboratory and the field. To predict the fate and transport of heavy metals from IBA leaching, a large-scale field trial study was performed using a big column (d × h = 3 m × 5.5 m) packed with 1-m thickness of IBA (approx. 10.6 tons) overlaid by 4-m sand layer. The determined field permeability (kF) was compared with that achieved from the laboratory, demonstrating a large disparity as much as 4 orders of magnitude likely due to IBA self-compaction. Indeed, back calculation using Blake-Kozeny's equation unveiled that, the “effective” diameters were significantly reduced by 21–46%. kF also demonstrated an anisotropic characteristic associated with fingered flows, trapped bubbles and heterogeneous consolidation/cementation efficiencies. To quantify the effects by kF, we ran a mechanistic model to simulate the transport of 11 heavy metals under advection (dh/dx = 0.05 m/m), indicating dramatically prolonged breakthrough time from days to centuries. Interestingly, breakthrough time was comparable among various metal ions (0–16.6% of RSD), suggesting their synchronous movements. Metal flux under kF was predicted in the end to address its toxicity potential, demonstrating limited environmental impacts in presence of the USEPA criterion.
AB - Permeability significantly affects leachate transportation. Yet, there often exists a gap for its measurements between laboratory and the field. To predict the fate and transport of heavy metals from IBA leaching, a large-scale field trial study was performed using a big column (d × h = 3 m × 5.5 m) packed with 1-m thickness of IBA (approx. 10.6 tons) overlaid by 4-m sand layer. The determined field permeability (kF) was compared with that achieved from the laboratory, demonstrating a large disparity as much as 4 orders of magnitude likely due to IBA self-compaction. Indeed, back calculation using Blake-Kozeny's equation unveiled that, the “effective” diameters were significantly reduced by 21–46%. kF also demonstrated an anisotropic characteristic associated with fingered flows, trapped bubbles and heterogeneous consolidation/cementation efficiencies. To quantify the effects by kF, we ran a mechanistic model to simulate the transport of 11 heavy metals under advection (dh/dx = 0.05 m/m), indicating dramatically prolonged breakthrough time from days to centuries. Interestingly, breakthrough time was comparable among various metal ions (0–16.6% of RSD), suggesting their synchronous movements. Metal flux under kF was predicted in the end to address its toxicity potential, demonstrating limited environmental impacts in presence of the USEPA criterion.
KW - Anisotropic
KW - Field permeability
KW - Heavy metals
KW - IBA leachate
KW - Transportation
UR - http://www.scopus.com/inward/record.url?scp=85074426638&partnerID=8YFLogxK
U2 - 10.1016/j.chemosphere.2019.125254
DO - 10.1016/j.chemosphere.2019.125254
M3 - Article
C2 - 31896190
AN - SCOPUS:85074426638
SN - 0045-6535
VL - 242
JO - Chemosphere
JF - Chemosphere
M1 - 125254
ER -